The ISOLDE (Isotope Separator On Line DEvice) Radioactive Ion Beam Facility, is an on-line isotope separator facility located at the centre of the CERN accelerator complex on the Franco-Swiss border. Created in 1964, the ISOLDE facility started delivering radioactive ion beams (RIBs) to users in 1967. Originally located at the synchro-cyclotron (SC) accelerator (CERN's first ever particle accelerator), the facility has been upgraded several times most notably in 1992 when the whole facility was moved to be connected to CERN's proton synchroton booster (PSB). ISOLDE is currently the longest-running facility in operation at CERN, with continuous developments of the facility and its experiments keeping ISOLDE at the forefront of science with RIBs. ISOLDE benefits a wide range of physics communities with applications covering nuclear, atomic, molecular and solid-state physics, but also biophysics and astrophysics, as well as high-precision experiments looking for physics beyond the Standard Model. The facility is operated by the ISOLDE Collaboration, comprising CERN and sixteen (mostly) European countries. As of 2019, close to 1,000 experimentalists around the world (including all continents) are coming to ISOLDE to perform typically 50 different experiments per year. Radioactive nuclei are produced at ISOLDE by shooting a high-energy (1.4GeV) beam of protons delivered by CERN's PSB accelerator on a 20 cm thick target. Several target materials are used depending on the desired final isotopes that are requested by the experimentalists. The interaction of the proton beam with the target material produces radioactive species through spallation, fragmentation and fission reactions. They are subsequently extracted from the bulk of the target material through thermal diffusion processes by heating the target to about 2,000 °C. The cocktail of produced isotopes is ultimately filtered using one of ISOLDE's two magnetic dipole mass separators to yield the desired isobar of interest. The time required for the extraction process to occur is dictated by the nature of the desired isotope and/or that of the target material and places a lower limit on the half-life of isotopes which can be produced by this method, and is typically of the order of a few milliseconds. For an additional separation, the Resonance Ionisation Laser Ion Source (RILIS) uses lasers to ionise a particular element, which separates the radioisotopes by their atomic number. Once extracted, the isotopes are directed either to one of several low-energy nuclear physics experiments or an isotope-harvesting area. A major upgrade of the REX post-accelerator to the HIE-ISOLDE (High Intensity and Energy Upgrade) superconducting linac completed construction in 2018, allowing for the re-acceleration of radioisotopes to higher energies than previously achievable.
Background Most atomic nuclei contain protons and neutrons. The number of protons determines the chemical element the nucleus belongs to. Different isotopes of the same element have different numbers of neutrons in their nuclei, but contain the same number of protons. For example, isotopes of carbon include carbon-12, carbon-13, carbon-14, which contain 6, 7, 8 neutrons respectively, but all contain 6 protons. Each isotope of an element has a different nuclear energy state, and may have different stability.
A nuclide is a more general term than isotope, and refers to atoms that have any particular number of protons and neutrons. Stable nuclides are not radioactive and do not spontaneously undergo radioactive decay, so are more usually found in nature. Whereas unstable (i.e. radioactive) nuclides are not found in nature, unless there is a recent source of them, because they are shorter lived, and will spontaneously decay, in one or more steps, to more stable nuclides. For example, carbon-14 is unstable but is found in nature. Scientists use accelerators and nuclear reactors to produce radioactive nuclides. As a general trend, and among other factors, the neutron–proton ratio of a nuclide determines its stability. The value of this ratio for stable nuclides generally increases for larger nuclei with more protons and neutrons. Many unstable nuclides have neutron-proton ratios beyond the zone of stability. The time required to lose half of a quantity of a given nuclide through radioactive decays, the half-life, is a measure of how stable an isotope is. Nuclides can be visually represented on a table (Segré chart or table of nuclides) where the proton number is plotted against the neutron number.
History
In 1950, two Danish physicists Otto Kofoed-Hansen and Karl-Ove Nielsen discovered a new technique for producing radioisotopes which enabled production of isotopes with shorter half-lives than earlier methods. The Copenhagen experiment they carried out included a simplified version of the same elements used in modern on-line experiments. Ten years later, in Vienna, at a symposium about separating radioisotopes, plans for an 'on-line' isotope separator were published. Using these plans, CERN's Nuclear Chemistry Group (NCG) built a prototype on-line mass separator coupled to target and ion source, which was bombarded by a 600 MeV proton beam delivered by CERN's the Synchro-Cyclotron. The test was a success and showed that the SC was an ideal machine for on-line rare isotope production. The plan for an electromagnetic isotope separator was developed during 1963–4 by European nuclear physicists and, in late 1964, their proposal was accepted by the CERN Director-General and the ISOLDE project began.
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